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[object Object], [object Object], [object Object] et al.

PLoS ONE • 2019

Microbial fuel cells (MFCs) can evolve in a viable technology if environmentally sound materials are developed and became available at low cost for these devices. This is especially important not only for the designing of large wastewater treatment systems, but also for the fabrication of low-cost, single-use devices. In this work we synthesized membranes by a simple procedure involving easily-biodegradable and economic materials such as poly (vinyl alcohol) (PVA), chitosan (CS) and the composite PVA:CS. Membranes were chemical and physically characterized and compared to Nafion®. Performance was studied using the membrane as separator in a typical H-Type MFCs showing that PVA:CS membrane outperform Nafion® 4 times (power production) while being 75 times more economic. We found that performance in MFC depends over interactions among several membrane characteristics such as oxygen permeability and ion conductivity. Moreover, we design a paper-based micro-scale MFC, which was used as a toxicity assay using 16 μL samples containing formaldehyde as a model toxicant. The PVA:CS membrane presented here can offer low environmental impact and become a very interesting option for point of need single-use analytical devices, especially in low-income countries where burning is used as disposal method, and toxic fluoride fumes (from Nafion®) can be released to the environment.

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International Journal of Renewable Energy Development • 2018

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[object Object], [object Object], [object Object] et al.

Fermentation • 2023

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[object Object], [object Object], [object Object] et al.

Water • 2023

[object Object], [object Object], [object Object] et al.

Toxics • 2022

[object Object], [object Object], [object Object] et al.

Frontiers in Microbiology • 2025

Microbial fuel cells (MFCs) have become one of the most promising technologies in the field of ecology and environmental science due to their dual functions of power generation and pollutant removal. However, the generally low power generation performance of MFCs is one of the bottlenecks constraining their development, and numerous studies have focused on the improvement of power generation performance. The majority of previous empirical studies were based on single experimental data, which means there may be large differences in experimental conditions and settings, leading to various or even contradictory conclusions. In this study, we collected a total of 10,826 cases from 186 publications in the China National Knowledge Infrastructure Database to quantitatively and systematically investigate the general patterns and driving factors of power generation performance in MFCs. Our results showed that (1) the power density, voltage, and reaction duration were significantly lower (~25%) in this study, while the coulombic efficiency and ambient temperature were significantly higher (13.4-33.1%) than those reported in other meta-analyses or review papers; (2) reaction chamber volume and cathode surface area were stronger predictors for the majority of power generation performance indices than other device configuration indices, especially cathode chamber volume, which explained >70% of the variances in power density and coulombic efficiency; (3) ambient temperature, external resistance, and reaction duration had greater effects on power generation performance than other reaction conditions; and (4) substrates with pre-treatment, especially with biological treatment, showed 10-40% higher values for the majority of power generation performance indices compared to pre-treatment with physical and chemical methods, and solid substrates showed better power generation performance than liquid and fluid substrates for the majority of indices. Our results suggest that dual-chamber systems, larger cathode surface areas, neutral pH levels, ambient temperatures of 30-35°C, and biological pre-treatment of substrates may be helpful in improving the power generation performance of MFCs.

[object Object], [object Object], [object Object] et al.

Renewable and Sustainable Energy Reviews • 2018

[object Object], [object Object], [object Object] et al.

Renewable and Sustainable Energy Reviews • 2018

Many factors affect the performance of microbial fuel cells (MFCs). Considerable attention has been given to the impact of cell configuration and materials on MFC performance. Much less work has been done on the impact of the anode microbiota, particularly in the context of using complex substrates as fuel. One strategy to improve MFC performance on complex substrates such as wastewater, is to pre-enrich the anode with known, efficient electrogens, such as Geobacter spp. The implication of this strategy is that the electrogens are the limiting factor in MFCs fed complex substrates and the organisms feeding the electrogens through hydrolysis and fermentation are not limiting. We conducted a systematic test of this strategy and the assumptions associated with it. Microbial fuel cells were enriched using three different substrates (acetate, synthetic wastewater and real domestic wastewater) and three different inocula (Activated Sludge, Tyne River sediment, effluent from an MFC). Reactors were either enriched on complex substrates from the start or were initially fed acetate to enrich for Geobacter spp. before switching to synthetic or real wastewater. Pre-enrichment on acetate increased the relative abundance of Geobacter spp. in MFCs that were switched to complex substrates compared to MFCs that had been fed the complex substrates from the beginning of the experiment (wastewater-fed MFCs - 21.9 ± 1.7% Geobacter spp.; acetate-enriched MFCs, fed wastewater - 34.9 ± 6.7% Geobacter spp.; Synthetic wastewater fed MFCs - 42.5 ± 3.7% Geobacter spp.; acetate-enriched synthetic wastewater-fed MFCs - 47.3 ± 3.9% Geobacter spp.). However, acetate pre-enrichment did not translate into significant improvements in cell voltage, maximum current density, maximum power density or substrate removal efficiency. Nevertheless, coulombic efficiency (CE) was higher in MFCs pre-enriched on acetate when complex substrates were fed following acetate enrichment (wastewater-fed MFCs - CE = 22.0 ± 6.2%; acetate-enriched MFCs, fed wastewater - CE =58.5 ± 3.5%; Synthetic wastewater fed MFCs - CE = 22.0 ± 3.2%; acetate-enriched synthetic wastewater-fed MFCs - 28.7 ± 4.2%.) The relative abundance of Geobacter ssp. and CE represents the average of the nine replicate reactors inoculated with three different inocula for each substrate. Efforts to improve the performance of anodic microbial communities in MFCs utilizing complex organic substrates should therefore focus on enhancing the activity of organisms driving hydrolysis and fermentation rather the terminal-oxidizing electrogens.

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[object Object], [object Object], [object Object] et al.

Advances in Microbiology • 2016

[object Object], [object Object], [object Object] et al.

Advanced Science • 2017

One of the challenges in Microbial Fuel Cell (MFC) technology is the improvement of the power output and the lowering of the cost required to scale up the system to reach usable energy levels for real life applications. This can be achieved by stacking multiple MFC units in modules and using cost effective ceramic as a membrane/chassis for the reactor architecture. The main aim of this work is to increase the power output efficiency of the ceramic based MFCs by compacting the design and exploring the ceramic support as the building block for small scale modular multi-unit systems. The comparison of the power output showed that the small reactors outperform the large MFCs by improving the power density reaching up to 20.4 W/m 3 (mean value) and 25.7 W/m 3 (maximum). This can be related to the increased surface-area-to-volume ratio of the ceramic membrane and a decreased electrode distance. The power performance was also influenced by the type and thickness of the ceramic separator as well as the total surface area of the anode electrode. The study showed that the larger anode electrode area gives an increased power output. The miniaturized design implemented in 560-units MFC stack showed an output up to 245 mW of power and increased power density. Such strategy would allow to utilize the energy locked in urine more efficiently, making MFCs more applicable in industrial and municipal wastewater treatment facilities, and scale-up-ready for real world implementation.

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[object Object], [object Object]

European Scientific Journal ESJ • 2020

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Constructed wetland-microbial fuel cells (CWL-MFCs) are eco-friendly and sustainable technology, simultaneously implementing contaminant removal and electricity production. According to intensive research over the last five years, this review on the operation mechanism was conducted for in-depth understanding and application guidance of CWL-MFCs. The electrochemical mechanism based on anodic oxidation and cathodic reduction is the core for improved treatment in CWL-MFCs compared to CWLs. As the dominant bacterial community, the abundance and gene-expression patterns of electro-active bacteria responds to electrode potentials and contaminant loadings, further affecting operational efficiency of CWL-MFCs. Plants benefit COD and N removal by supplying oxygen for aerobic degradation and rhizosphere secretions for microorganisms. Multi-electrode configuration, carbon-based electrodes and rich porous substrates affect transfer resistance and bacterial communities. The possibilities of CWL-MFCs targeting at recalcitrant contaminants like flame retardants and interchain interactions among effect components need systematic research.

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[object Object], [object Object], [object Object] et al.

Journal of Xenobiotics • 2025

Over the past few decades, there has been a growing concern regarding the fate and transport of pharmaceuticals, particularly antibiotics, as emerging contaminants in the environment. It has been proposed that the presence of antibiotics at concentrations typically found in wastewater can impact the dynamics of bacterial populations and facilitate the spread of antibiotic resistance. The efficiency of currently-used wastewater treatment technologies in eliminating pharmaceuticals is often insufficient, resulting in the release of low concentrations of these compounds into the environment. In this study, we addressed these challenges by evaluating how different influent ibuprofen (IBU) concentrations influenced the efficiency of a laboratory-scale, integrated constructed wetland-microbial fuel cell (CW-MFC) system seeded with Eichhornia crassipes , in terms of organic matter removal, electricity generation, and change of bacterial community structure compared to unplanted, sediment MFC (S-MFC) and abiotic S-MFC (AS-MFC). We observed that the addition of IBU (5 mg L -1 ) resulted in a notable decrease in chemical oxygen demand (COD) and electricity generation, suggesting that high influent IBU concentrations caused partial inhibition for the electroactive microbial community due to its complexity and aromaticity. However, CW-MFC could recover from IBU inhibition after an acclimation period compared to unplanted S-MFC, even though the influent IBU level was increased up to 20 mg L -1 , suggesting that plants in CW-MFCs have a beneficial role in relieving the inhibition of anode respiration due to the presence of high levels of IBU; thus, promoting the metabolic activity of the electroactive microbial community. Similarly, IBU removal efficiency for CW-MFC ( i.e. , 49-62%) was much higher compared to SMFC ( i.e. , 29-42%), and AS-MFC ( i.e. , 20-22%) during all experimental phases. In addition, our high throughput sequencing revealed that the high performance of CW-MFCs compared to S-MFC was associated with increasing the relative abundances of several microbial groups that are closely affiliated with anode respiration and organic matter fermentation. In summary, our results show that the CW-MFC system demonstrates suitability for high removal efficiency of IBU and effective electricity generation.